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Compelling evidence in Sub-Saharan Africa (SSA) shows that Climate-Smart Agriculture (CSA) has a positive impact on agricultural productivity. However, the uptake of CSA remains low, which is related to anthropogenic, or human-related, decisions about CSA and agricultural land use. This paper assesses households’ decisions to allocate agricultural land to CSA technologies across space and over time. We use the state-contingent theory, mixed methods, and mixed data sources. While agricultural land is increasing, forest land is decreasing across countries in SSA. The results show that household decisions to use CSA and the extent of agricultural land allocation to CSA remain low with a negative trend over time in SSA. Owned land and accessing land through rental markets are positively associated with allocating land to CSA technologies, particularly where land pressure is high. Regarding adaptation, experiencing rainfall shocks is significantly associated with anthropogenic land allocation to CSA technologies. The country policy assessment further supports the need to scale up CSA practices for adaptation, food security, and mitigation. Therefore, scaling up CSA in SSA will require that agriculture-related policies promote land tenure security and land markets while promoting climate-smart farming for food security, adaptation, and mitigation.